Low-temperature hysteresis broadening emerging from domain-wall creep dynamics in a two-phase competing system

Autor: Keisuke Matsuura, Yo Nishizawa, Yuto Kinoshita, Takashi Kurumaji, Atsushi Miyake, Hiroshi Oike, Masashi Tokunaga, Yoshinori Tokura, Fumitaka Kagawa
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: Communications Materials, Vol 4, Iss 1, Pp 1-8 (2023)
Druh dokumentu: article
ISSN: 2662-4443
DOI: 10.1038/s43246-023-00399-8
Popis: Abstract Hysteretic behaviour accompanies any first-order phase transition, forming a basis for many applications. However, its quantitative understanding remains challenging, and even a qualitative understanding of pronounced hysteresis broadening at low temperature, which is often observed in magnetic-field-induced first-order phase transition materials, is unclear. Here, we show that such pronounced hysteresis broadening emerges if the phase-front velocity during the first-order phase transition exhibits an activated behaviour as a function of both temperature and magnetic field. This is demonstrated by using real-space magnetic imaging techniques, for the magnetic-field-induced first-order phase transition between antiferromagnetic and ferrimagnetic phases in (Fe0.95Zn0.05)2Mo3O8. When combined with the Kolmogorov-Avrami-Ishibashi model, the observed activated temperature- and field-dependences of the growth velocity of the emerging antiferromagnetic domain quantitatively reproduce the pronounced hysteresis broadening. Furthermore, the same approach also reproduces the field-sweep-rate dependence of the transition field observed in the experiment. Our findings thus provide a quantitative and comprehensive understanding of pronounced hysteresis broadening from the microscopic perspective of domain growth.
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