A Nitrogen‐Doped Porous Carbon Supported Copper Catalyst from a Scalable One‐Step Method for Efficient Carbon Dioxide Electroreduction

Autor:	Dr. Amruthalakshmi Vijayakumar, Dr. Yong Zhao, Dr. Kezhong Wang, Dr. Yunfeng Chao, Prof. Haiqun Chen, Prof. Caiyun Wang, Prof. Gordon G. Wallace
Jazyk:	angličtina
Rok vydání:	2023
Předmět:	Carbon Dioxide Reduction Electrocatalyst Copper Nanoparticles C1 products N-Doped Carbon Industrial electrochemistry TP250-261 Chemistry QD1-999
Zdroj:	ChemElectroChem, Vol 10, Iss 2, Pp n/a-n/a (2023)
Druh dokumentu:	article
ISSN:	2196-0216 20220081
DOI:	10.1002/celc.202200817
Popis:	Abstract In this work, a scalable one‐step glucose blowing method has been used to prepare a porous N‐doped carbon supported Cu nanoparticles (Cu‐NC) composite catalyst for CO2 electroreduction. This Cu‐NC catalyst demonstrates efficient catalytic activity for CO2‐to‐C1 product (CO and formate) conversion, with a high efficiency of 69 % at an overpotential of 590 mV. The excellent catalytic activity is correlated to the structure of this composite and the N‐species (pyridinic and graphitic nitrogen) in the carbonaceous matrix that may promote the CO2 adsorption and subsequent formation of reduction reaction intermediates and products.
Databáze:	Directory of Open Access Journals
Externí odkaz:	https://doaj.org/article/f7a43cf437254f52ba36bf5715077417 Zobrazit plný text záznamu Plný text View record in DOAJ