Growth of ultimate high-density scintillating films for high-resolution X-ray imaging at synchrotrons

Autor: Laura Wollesen, Paul-Antoine Douissard, Philip Cook, Pavel Loiko, Gurvan Brasse, Jérémie Margueritat, Patrice Camy, Thierry Martin, Christophe Dujardin
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Optical Materials: X, Vol 22, Iss , Pp 100309- (2024)
Druh dokumentu: article
ISSN: 2590-1478
DOI: 10.1016/j.omx.2024.100309
Popis: Scintillators are X-ray to visible light converters applied in X-ray imaging detectors used at synchrotrons. Drastically improved performances of the 4th generation synchrotron sources enable us to perform X-ray imaging experiments at higher energies. For high spatial resolution X-ray imaging (micrometer to submicrometer), thin scintillating films are required. Consequently, especially for high X-ray energies (30keV to 100keV), the detection efficiency is limited due to the low X-ray absorption efficiency of the thin films. We have used Liquid Phase Epitaxy (LPE) to grow thin films of one of the ultimate high-density materials, Lu2Hf2O7:Eu3+, which demonstrate scintillating properties and thus combine high spatial resolution and maximized absorption efficiency. X-ray imaging experiments demonstrate that the Modulation Transfer Function (MTF) reaches 10% at 900 lp/mm, and radiographs visually confirm the promising imaging properties. We present structural, luminescent, and scintillation characterization of Lu2Hf2O7:Eu thin films grown on ZrO2:Y substrates, showing that the films crystallize in the disordered fluorite structure and the europium ions incorporate into the structure and enhance the luminescence intensity. This contribution is a first step toward developing promising ultra-dense, hafnate-based scintillating screens for high spatial resolution X-ray imaging.
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