Apportionment and Inventory Optimization of Agriculture and Energy Sector Methane Emissions Using Multi‐Month Trace Gas Measurements in Northern Colorado

Autor: Griffin J. Mead, Daniel I. Herman, Fabrizio R. Giorgetta, Nathan A. Malarich, Esther Baumann, Brian R. Washburn, Nathan R. Newbury, Ian Coddington, Kevin C. Cossel
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Geophysical Research Letters, Vol 51, Iss 2, Pp n/a-n/a (2024)
Druh dokumentu: article
ISSN: 1944-8007
0094-8276
DOI: 10.1029/2023GL105973
Popis: Abstract Quantifying sector‐resolved methane fluxes in complex emissions environments is challenging yet necessary to improve emissions inventories and guide policy. Here, we separate energy and agriculture sector emissions using a dynamic linear model analysis of methane, ethane, and ammonia data measured at a Northern Colorado site from November 2021 to January 2022. By combining these sector‐apportioned observations with spatially resolved inventories and Bayesian inverse methods, energy and agriculture methane fluxes are optimized across the study's ∼850 km2 sensitivity area. Energy sector fluxes are synthesized with previous literature to evaluate trends in energy sector methane emissions. Optimized agriculture fluxes in the study area were 3.5× larger than inventory estimates; we demonstrate this discrepancy is consistent with differences in the modeled versus real‐world spatial distribution of agricultural sources. These results highlight how sector‐apportioned methane observations can yield multi‐sector inventory optimizations in complex environments.
Databáze: Directory of Open Access Journals