Sea Spray Aerosol Over the Remote Oceans Has Low Organic Content

Autor: Michael J. Lawler, Gregory P. Schill, Charles A. Brock, Karl D. Froyd, Christina Williamson, Agnieszka Kupc, Daniel M. Murphy
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: AGU Advances, Vol 5, Iss 4, Pp n/a-n/a (2024)
Druh dokumentu: article
ISSN: 2576-604X
DOI: 10.1029/2024AV001215
Popis: Abstract Biogenic organic compounds in the surface ocean may significantly alter the cloud‐forming ability of sea spray aerosol and thereby affect the amount of solar radiation reaching the ocean surface. Estimates of the organic mass fraction of sea spray vary widely, and some results show a significant dependence on biological activity in the source seawater. We present airborne observations of the organic mass fraction of individual sea spray particles measured using the Particle Analysis by Laser Mass Spectrometry (PALMS) instrument during the Atmospheric Tomography (ATom) mission, which sampled a wide range of latitudes and altitudes over the remote Atlantic and Pacific Oceans across four seasons, from the marine boundary layer to the upper troposphere. The measured sea spray particles of about 0.15–0.7 μm dry diameter showed higher average organic mass fractions at smaller sizes, but values were low overall, with regional integrated submicron means almost always
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