| Autor: |
Ju Huang, Zhiyuan Zhang, Yuxue Wei, Lisheng Guo, Jiuyi Liu, Chenghua Zhang, Zhaoming Xue, Song Sun |
| Jazyk: |
angličtina |
| Rok vydání: |
2023 |
| Předmět: |
|
| Zdroj: |
Chemistry of Inorganic Materials, Vol 1, Iss , Pp 100004- (2023) |
| Druh dokumentu: |
article |
| ISSN: |
2949-7469 |
| DOI: |
10.1016/j.cinorg.2023.100004 |
| Popis: |
CO2 hydrogenation to yield long-chain hydrocarbons has attracted tremendous attention in both academic and industrial field. CuFe-based bimetal catalysts have been widely applied in CO2 hydrogenation owing to their low cost, facile preparation, and excellent performance. In this study, a series of CuFe-based catalysts with different Cu/Fe molar ratios have been synthesized from layered double hydroxide precursor. The optimized CuFe8-LDO catalyst with Cu:Fe=1:8 exhibits a C5+ selectivity of 45% at CO2 conversion of 9.5%. Through systematic characterizations including TEM, TPR, TPD, XPS, it is revealed the abundant and highly dispersed CuO favors the reduction of iron species, and enhances CO adsorption capacity of as-prepared catalysts. This study provides an in-deep understanding of Cu on CO2 hydrogenation performance of Fe-based catalysts. |
| Databáze: |
Directory of Open Access Journals |
| Externí odkaz: |
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