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Abstract Soft materials that convert light into mechanical energy can create new untethered strategies for actuating soft robotics. Yet, the available light‐driven materials are often incompatible with standard fabrication in soft robotics and restricted to shapes (e.g., sheets) that have limited capability for 3D deformation; often laser or focused light is required for actuation. Here, to address these challenges, a straightforward method for synthesizing sunlight‐responsive fluidic actuators from off‐the‐shelf silicone precursors capable of expanding in 3D is developed. A liquid phase and activated carbon as photothermal elements are constrained in the elastomer. Solar spectral light triggers a liquid–gas phase transition creating sufficient pressure to overcome the internal elastic stress and actuate the material. The fluidic actuation is characterized under varying light conditions reaching expansion cycle times between ≈20–500 s, strains of 28%, and actuation stress of ≈1.3 MPa in different experiments. The materials were then used to exemplarily drive a mechanical switch, a liquid dispensing soft pump, a valve, and a bending actuator. As the described materials are easy to produce in a 5 min synthesis by standard molding techniques, it is believed that they are a promising opportunity for embodied energy converters in environmentally powered soft robots that respond to sunlight. |
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