Autor: |
Inhee Maeng, Asuka Matsuyama, Jung-Ho Yun, Shenghao Wang, Chul Kang, Chul-Sik Kee, Masakazu Nakamura, Min-Cherl Jung |
Jazyk: |
angličtina |
Rok vydání: |
2020 |
Předmět: |
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Zdroj: |
Nanomaterials, Vol 10, Iss 4, p 721 (2020) |
Druh dokumentu: |
article |
ISSN: |
2079-4991 |
DOI: |
10.3390/nano10040721 |
Popis: |
To control the density of a CH3NH2 molecular defect, which strongly contributed to a significant THz-wave absorption property in the CH3NH3PbI3 hybrid perovskite thin film formed by the sequential vacuum evaporation method, we performed post-annealing processes with various temperatures and times. In the thin film after post-annealing at 110 °C for 45 min, the density of the CH3NH2 molecular defect was minimized, and CH3NH3I and PbI2 disappeared in the thin film after the post-annealing process at 150 °C for 30 min. However, the density of the CH3NH2 molecular defect increased. Moreover, the THz-wave absorption property for each thin film was obtained using a THz time-domain spectroscopy to understand the correlation between the density of a molecular defect and the THz-wave oscillation strength at 1.6 THz, which originated in the molecular defect-incorporated hybrid perovskite structure. There is a strong linear correlation between the oscillator strength of a significant THz-wave absorption at 1.6 THz and the CH3NH2 molecular defect density. |
Databáze: |
Directory of Open Access Journals |
Externí odkaz: |
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