A vacuum ultraviolet laser with a submicrometer spot for spatially resolved photoemission spectroscopy

Autor: Yuanhao Mao, Dong Zhao, Shen Yan, Hongjia Zhang, Juan Li, Kai Han, Xiaojun Xu, Chuan Guo, Lexian Yang, Chaofan Zhang, Kun Huang, Yulin Chen
Jazyk: angličtina
Rok vydání: 2021
Předmět:
Zdroj: Light: Science & Applications, Vol 10, Iss 1, Pp 1-8 (2021)
Druh dokumentu: article
ISSN: 2047-7538
DOI: 10.1038/s41377-021-00463-3
Popis: Abstract Vacuum ultraviolet (VUV) lasers have demonstrated great potential as the light source for various spectroscopies, which, if they can be focused into a small beam spot, will not only allow investigation of mesoscopic materials and structures but also find application in the manufacture of nano-objects with excellent precision. In this work, we report the construction of a 177 nm VUV laser that can achieve a record-small (~0.76 μm) focal spot at a long focal length (~45 mm) by using a flat lens without spherical aberration. The size of the beam spot of this VUV laser was tested using a metal grating and exfoliated graphene flakes, and we demonstrated its application in a fluorescence spectroscopy study on pure and Tm3+-doped NaYF4 microcrystals, revealing a new emission band that cannot be observed in the traditional up-conversion process. In addition, this laser system would be an ideal light source for spatially and angle-resolved photoemission spectroscopy.
Databáze: Directory of Open Access Journals