Topologically enhanced nonlinear optical response of graphene nanoribbon heterojunctions

Autor: Hanying Deng, Zhihao Qu, Yingji He, Changming Huang, Nicolae C. Panoiu, Fangwei Ye
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: Quantum Frontiers, Vol 2, Iss 1, Pp 1-9 (2023)
Druh dokumentu: article
ISSN: 2731-6106
DOI: 10.1007/s44214-023-00036-y
Popis: Abstract We study the nonlinear optical properties of heterojunctions made of graphene nanoribbons (GNRs) consisting of two segments with either the same or different topological properties. By utilizing a quantum mechanical approach that incorporates distant-neighbor interactions, we demonstrate that the presence of topological interface states significantly enhances the second- and third-order nonlinear optical response of GNR heterojunctions that are created by merging two topologically inequivalent GNRs. Specifically, GNR heterojunctions with topological interface states display third-order harmonic hyperpolarizabilities that are more than two orders of magnitude larger than those of their similarly sized counterparts without topological interface states, whereas the second-order harmonic hyperpolarizabilities exhibit a more than ten-fold contrast between heterojunctions with and without topological interface states. Additionally, we find that the topological state at the interface between two topologically distinct GNRs can induce a noticeable red-shift of the quantum plasmon frequency of the heterojunctions. Our results reveal a general and profound connection between the existence of topological states and an enhanced nonlinear optical response of graphene nanostructures and possible other photonic systems.
Databáze: Directory of Open Access Journals
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