Autor: |
Hanying Deng, Zhihao Qu, Yingji He, Changming Huang, Nicolae C. Panoiu, Fangwei Ye |
Jazyk: |
angličtina |
Rok vydání: |
2023 |
Předmět: |
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Zdroj: |
Quantum Frontiers, Vol 2, Iss 1, Pp 1-9 (2023) |
Druh dokumentu: |
article |
ISSN: |
2731-6106 |
DOI: |
10.1007/s44214-023-00036-y |
Popis: |
Abstract We study the nonlinear optical properties of heterojunctions made of graphene nanoribbons (GNRs) consisting of two segments with either the same or different topological properties. By utilizing a quantum mechanical approach that incorporates distant-neighbor interactions, we demonstrate that the presence of topological interface states significantly enhances the second- and third-order nonlinear optical response of GNR heterojunctions that are created by merging two topologically inequivalent GNRs. Specifically, GNR heterojunctions with topological interface states display third-order harmonic hyperpolarizabilities that are more than two orders of magnitude larger than those of their similarly sized counterparts without topological interface states, whereas the second-order harmonic hyperpolarizabilities exhibit a more than ten-fold contrast between heterojunctions with and without topological interface states. Additionally, we find that the topological state at the interface between two topologically distinct GNRs can induce a noticeable red-shift of the quantum plasmon frequency of the heterojunctions. Our results reveal a general and profound connection between the existence of topological states and an enhanced nonlinear optical response of graphene nanostructures and possible other photonic systems. |
Databáze: |
Directory of Open Access Journals |
Externí odkaz: |
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