Cooling dynamics of electrons in MAPbBr3 probed in the deep-UV

Autor: Rossi Thomas Charles, Wang Lijie, Oppermann Malte, Chen Peter, Chiang Yu-Hsien, Tsai Ming-Chang, Shih Chun-Hua, Guo Tsung-Fang, Chergui Majed
Jazyk: angličtina
Rok vydání: 2019
Předmět:
Zdroj: EPJ Web of Conferences, Vol 205, p 05020 (2019)
Druh dokumentu: article
ISSN: 2100-014X
DOI: 10.1051/epjconf/201920505020
Popis: Transient absorption in the Visible and in the deep-UV is performed on MAPbBr3 thin films with 3.1 eV pump excitation. The UV probe can access higher order transitions in the material exploring different high-symmetry points of the Brillouin zone. Uncorrelated electron-hole pairs are generated within the instrument response function of 150 fs. The photobleaching at 3.3 eV shows that electron cooling happens in ~ 1 ps.
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