| Autor: |
Ru Han, Linlin Chen, Bohang Xing, Qiangsheng Guo, Jindan Tian, Na Sha, Zhe Zhao |
| Jazyk: |
angličtina |
| Rok vydání: |
2022 |
| Předmět: |
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| Zdroj: |
Catalysis Communications, Vol 165, Iss , Pp 106440- (2022) |
| Druh dokumentu: |
article |
| ISSN: |
1873-3905 |
| DOI: |
10.1016/j.catcom.2022.106440 |
| Popis: |
In this study, a transition metal-based perovskite oxide catalyst with high CH3OH yield was successfully developed. The A-site substitution by Pr3+ in La1-xPrxMn0.6Ni0.4O3-δ can effectively adjust the activity of the perovskite catalysts for the direct conversion of CO2 and H2O into hydrocarbon fuels, especially CH3OH. Based on the designed photo-thermo synergetic photosynthesis strategy, the first hour CH3OH yield of La1-xPrxMn0.6Ni0.4O3-δ reached 3.97 mmol g−1, while only 0.24 μmol g−1 under normal photocatalysis mode. The synergistic photo-thermo catalysis was demonstrated to be a promising strategy for the future artificial photosynthesis development. |
| Databáze: |
Directory of Open Access Journals |
| Externí odkaz: |
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