Charge-separation driven mechanism via acylium ion intermediate migration during catalytic carbonylation in mordenite zeolite

Autor: Wei Chen, Karolina A. Tarach, Xianfeng Yi, Zhiqiang Liu, Xiaomin Tang, Kinga Góra-Marek, Anmin Zheng
Jazyk: angličtina
Rok vydání: 2022
Předmět:
Zdroj: Nature Communications, Vol 13, Iss 1, Pp 1-13 (2022)
Druh dokumentu: article
ISSN: 2041-1723
DOI: 10.1038/s41467-022-34708-5
Popis: The tremendous application of carbonylation reaction requires the elaborate explanation to reaction mechanism. Here the authors propose a charge-separation driven mechanism of methyl acetate formation via acylium ion intermediate in mordenite zeolite by an integrated reaction/diffusion kinetics model during the dimethyl ether carbonylation.
Databáze: Directory of Open Access Journals