A laser-ARPES study of LaNiO3 thin films grown by sputter deposition

Autor: Edoardo Cappelli, Willem O. Tromp, Siobhan McKeown Walker, Anna Tamai, Marta Gibert, Felix Baumberger, Flavio Y. Bruno
Jazyk: angličtina
Rok vydání: 2020
Předmět:
Zdroj: APL Materials, Vol 8, Iss 5, Pp 051102-051102-6 (2020)
Druh dokumentu: article
ISSN: 2166-532X
DOI: 10.1063/1.5143316
Popis: Thin films of the correlated transition-metal oxide LaNiO3 undergo a metal–insulator transition when their thickness is reduced to a few unit cells. Here, we use angle-resolved photoemission spectroscopy to study the evolution of the electronic structure across this transition in a series of epitaxial LaNiO3 films of thicknesses ranging from 19 u.c. to 2 u.c. grown in situ by RF magnetron sputtering. Our data show a strong reduction in the electronic mean free path as the thickness is reduced below 5 u.c. This prevents the system from becoming electronically two-dimensional, as confirmed by the largely unchanged Fermi surface seen in our experiments. In the insulating state, we observe a strong suppression of the coherent quasiparticle peak, but no clear gap. These features resemble previous observations of the insulating state of NdNiO3.
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