Probing the local nature of excitons and plasmons in few-layer MoS2

Autor: Hannah Catherine Nerl, Kirsten Trøstrup Winther, Fredrik S. Hage, Kristian Sommer Thygesen, Lothar Houben, Claudia Backes, Jonathan N. Coleman, Quentin M. Ramasse, Valeria Nicolosi
Jazyk: angličtina
Rok vydání: 2017
Předmět:
Zdroj: npj 2D Materials and Applications, Vol 1, Iss 1, Pp 1-9 (2017)
Druh dokumentu: article
ISSN: 2397-7132
DOI: 10.1038/s41699-017-0003-9
Popis: Probing excitons and plasmons at the nanoscale This paper outlines a template protocol to map the local nature of electronic excitations were they happen, at the nanoscale. An unprecedented combination of energy and spatial resolution (using monochromated low-loss scanning-transmission-electron-microscopy electron-energy-loss spectroscopy) was used to map for the first time local electronic excitations of 2D nanomaterials. These are crucially important to understand and explain any type of opto-electronic behaviour in 2D materials. Using this cutting-edge technique combined with a computational approach we were able to unravel the full set of electronic excitations (plasmonic and excitonic) in MoS2 nanosheets over a wide energy range. This study will be important for the application of nanomaterials for realistic applications in opto-electronics.
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