The Synthesis of Functionalized Carbonized Polymer Dots via Reversible Assembly of Oligomers for Anti‐Counterfeiting, Catalysis, and Gas storage

Autor: Yu Wang, Yingxi Qin, Fengya Wang, Hongyu Zhang, Changxin Huangfu, Yushu Shi, Xize Chen, Zhenming Wang, Wenming Tian, Liang Feng
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Advanced Science, Vol 11, Iss 38, Pp n/a-n/a (2024)
Druh dokumentu: article
ISSN: 2198-3844
DOI: 10.1002/advs.202405043
Popis: Abstract Carbonized polymer dots (CPDs) have shown exceptional potential across a wide range of applications. However, their practical utilization is significantly greatly impeded by the lack of precise control over their structures and functionalities. Consequently, the development of controlled synthesis strategies for CPDs with well‐defined structures and tailored functionalities remains a critical challenge in the field. Here, the controlled synthesis of functional CPDs with reversible assembly properties via airflow‐assisted melt polymerization, followed by a one‐step post‐synthetic doping strategy, is reported. This synthetic approach achieves high product yield, uniform and tunable structures, as well as customized functionalities including solid‐state emission, enhanced catalytic performance (3.5–45 times higher than conventional methods), and selective gas storage in the resulting CPDs. The ability to tailor the properties of CPDs through controlled synthesis opens up new opportunities for their practical application in photocatalysis and gas storage.
Databáze: Directory of Open Access Journals
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