Collapse of metallicity and high-T c superconductivity in the high-pressure phase of FeSe0.89S0.11

Autor: Pascal Reiss, Alix McCollam, Zachary Zajicek, Amir A. Haghighirad, Amalia I. Coldea
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: npj Quantum Materials, Vol 9, Iss 1, Pp 1-9 (2024)
Druh dokumentu: article
ISSN: 2397-4648
DOI: 10.1038/s41535-024-00677-9
Popis: Abstract We investigate the high-pressure phase of the iron-based superconductor FeSe0.89S0.11 using transport and tunnel diode oscillator studies using diamond anvil cells. We construct detailed pressure-temperature phase diagrams that indicate that the superconducting critical temperature is strongly enhanced by more than a factor of four towards 40 K above 4 GPa. The resistivity data reveal signatures of a fan-like structure of non-Fermi liquid behaviour which could indicate the existence of a putative quantum critical point buried underneath the superconducting dome around 4.3 GPa. With further increasing the pressure, the zero-field electrical resistivity develops a non-metallic temperature dependence and the superconducting transition broadens significantly. Eventually, the system fails to reach a fully zero-resistance state, and the finite resistance at low temperatures becomes strongly current-dependent. Our results suggest that the high-pressure, high-T c phase of iron chalcogenides is very fragile and sensitive to uniaxial effects of the pressure medium, cell design and sample thickness. This high-pressure region could be understood assuming a real-space phase separation caused by nearly concomitant electronic and structural instabilities.
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