Geochemical modeling of changes in caprock permeability caused by CO2–brine–rock interactions under the diffusion mechanism

Autor: Ma Xin, Yang Guodong, Li Xufeng, Yu Ying, Dong Jianxing
Jazyk: English<br />French
Rok vydání: 2019
Předmět:
Zdroj: Oil & Gas Science and Technology, Vol 74, p 83 (2019)
Druh dokumentu: article
ISSN: 1294-4475
1953-8189
DOI: 10.2516/ogst/2019055
Popis: Geologic Carbon Sequestration (GCS) has been widely considered as a significant means for reducing CO2 emissions to address global climate change. The caprock sealing plays a key role in determining permanence and security of carbon dioxide (CO2) storage in geologic formations. This study presents geochemical modeling of CO2–brine–rock interactions in a deep saline aquifer in the Jianghan Basin, which is a potential target for CO2 injection and geological storage. A one-dimensional model was developed to investigate the changes in caprock permeability caused by CO2–brine–rock interactions under the diffusion mechanism. The results show that the dissolution of K-feldspar and albite plays a key role in the variation of caprock permeability, which makes permeability increased by 60% at the bottom of caprock. The caprock permeability is increased with temperature by enhancing the minerals dissolution of caprocks. In addition, the common-ion effect generated by the increased salinity inhibits the minerals dissolution in caprock.
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