| Autor: |
M. Saravanan, Rajkumar Palanisamy, V. Sethuraman, K. Diwakar, P. Senthil Kumar, P. Sundara Venkatesh, N. Kannan, R. Joel Kingston, K. Aravinth, Jinho Kim |
| Jazyk: |
angličtina |
| Rok vydání: |
2023 |
| Předmět: |
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| Zdroj: |
Energies, Vol 16, Iss 7, p 3286 (2023) |
| Druh dokumentu: |
article |
| ISSN: |
1996-1073 |
| DOI: |
10.3390/en16073286 |
| Popis: |
Increasing concerns about the vulnerability of the world’s energy supply and the necessity to implement sustainable technologies have prompted researchers to develop high-performance electrocatalysts that are affordable and efficient for converting and storing renewable energy. This article reports a facile approach to fabricating two-dimensional (2D) Ge-decorated h-BN/MoS2 heterostructure nanosheets by self-assembly for multiple electrochemical applications such as supercapacitor and hydrogen evolution reactions. The organization of the physical and chemical links between the germanium modulations on the heterostructure of boron nitride/molybdenum sulphide (Ge/h-BN/MoS2) were facilitated to generate more active sites. Furthermore, the asymmetric supercapacitor of Ge-decorated h-BN/MoS2 amplified the capacitance to 558.53 F g−1 at 1 A g−1 current density and 159.19 F g−1 at 10 A g−1, in addition to a retention rate of 85.69% after 2000 cycles. Moreover, the Ge-decorated h-BN/MoS2 catalyst realized a low over-potential value, with an RHE of 0.57 (HER) at 5 mA/cm2, a Tafel value of ∼204 mV/dec, and long-term electrolysis stability of 10 h. This work may open the door for further investigations on metal-decorated heterostructures, which have a significant potential for both supercapacitor and water-splitting applications. |
| Databáze: |
Directory of Open Access Journals |
| Externí odkaz: |
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