Improved performance of polymer light-emitting diodes using graphene oxide doped with silver nanoparticles as the hole-transport layer

Autor: Cheng-Liang Huang, Kuan-Ming Chen, Bo-Yuan Lu, Sy-Hann Chen
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: Results in Physics, Vol 55, Iss , Pp 107190- (2023)
Druh dokumentu: article
ISSN: 2211-3797
DOI: 10.1016/j.rinp.2023.107190
Popis: This study successfully demonstrates the fabrication of a thin film of graphene oxide doped with silver nanoparticles (GO:AgNPs) using electrochemical exfoliation and photochemical synthesis. The GO:AgNPs thin film exhibits a higher work function and conductivity compared to poly[3,4-ethylenedioxythiophene] polystyrene sulfonate (PEDOT:PSS), making it a promising candidate for the hole-transport layer in polymer light-emitting diodes (PLEDs). Among various configurations, a PLED incorporating GO:AgNPs as the interlayer, which is prepared under blue-light illumination, exhibits optimal luminescent performance. This configuration achieves the highest luminance of 6341 cd/m2 and the highest average current efficiency of 1.87 cd/A. Notably, this novel PLED demonstrates a remarkable 168 % enhancement in average current efficiency and an impressive 637 % increase in electroluminescence intensity compared to a PLED employing a PEDOT:PSS interlayer.
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