Photocatalytic degradation of paracetamol on immobilized TiO2 in a low-tech reactor by solar light for water treatment

Autor: Lukas Dufner, Lluc Aresté-Saló, Moisès Graells, Montserrat Pérez-Moya, Frank Kern, Wolfgang Rheinheimer
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Open Ceramics, Vol 18, Iss , Pp 100599- (2024)
Druh dokumentu: article
ISSN: 2666-5395
DOI: 10.1016/j.oceram.2024.100599
Popis: Photocatalytic water treatment is an appealing concept to mineralize organic contaminants in contaminated water. In this study, the UV-resistant drug paracetamol (PCT) in aqueous solution is degraded by using a solar irradiated loop-reactor equipped with a TiO2 (P25) photocatalyst. The catalyst powder was dispersed in a geopolymer surface coating applied to aluminum-U-profiles connected by filament-printed polymer elements. Different assays with variations in initial PCT concentration were performed under natural solar radiation to determine the degradation kinetics of the PCT and correlate it to applied solar radiation energy density. Depending on experimental conditions, degradation efficiencies of 37.0–75.1 % were achieved within 3 h. Control samples without catalyst show no degradation. No degradation of the catalyst activity was observed within 42 h of operation time. The study shows the feasibility of this simple and scalable reactor design and coating technology for water purification under off-grid conditions provided sufficient solar radiation is available.
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