Steering the reaction pathway of syngas-to-light olefins with coordination unsaturated sites of ZnGaOx spinel

Autor: Na Li, Yifeng Zhu, Feng Jiao, Xiulian Pan, Qike Jiang, Jun Cai, Yifan Li, Wei Tong, Changqi Xu, Shengcheng Qu, Bing Bai, Dengyun Miao, Zhi Liu, Xinhe Bao
Jazyk: angličtina
Rok vydání: 2022
Předmět:
Zdroj: Nature Communications, Vol 13, Iss 1, Pp 1-8 (2022)
Druh dokumentu: article
ISSN: 2041-1723
DOI: 10.1038/s41467-022-30344-1
Popis: Great progress has been made in the development of bifunctional oxide-zeolite catalysts to tackle the selectivity challenge in syngas chemistry. Here the authors show syngas conversion can be steered along a highly active and selective pathway towards light olefins via ketene acetate (acetyl) intermediates.
Databáze: Directory of Open Access Journals