Estimation of Canada's methane emissions: inverse modelling analysis using the Environment and Climate Change Canada (ECCC) measurement network

Autor: M. Ishizawa, D. Chan, D. Worthy, E. Chan, F. Vogel, J. R. Melton, V. K. Arora
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Atmospheric Chemistry and Physics, Vol 24, Pp 10013-10038 (2024)
Druh dokumentu: article
ISSN: 1680-7316
1680-7324
DOI: 10.5194/acp-24-10013-2024
Popis: Canada has major sources of atmospheric methane (CH4), with the world's second-largest boreal wetland and the world's fourth-largest natural gas production. However, Canada's CH4 emissions remain uncertain among estimates. Better quantification and characterization of Canada's CH4 emissions are critical for climate mitigation strategies. To improve our understanding of Canada's CH4 emissions, we performed an ensemble regional inversion for 2007–2017 constrained with the Environment and Climate Change Canada (ECCC) surface measurement network. The decadal CH4 estimates show no significant trend, unlike some studies that reported long-term trends. The total CH4 estimate is 17.4 (15.3–19.5) Tg CH4 yr−1, partitioned into natural and anthropogenic sources at 10.8 (7.5–13.2) and 6.6 (6.2–7.8) Tg CH4 yr−1, respectively. The estimated anthropogenic emission is higher than inventories, mainly in western Canada (with the fossil fuel industry). Furthermore, the results reveal notable spatiotemporal characteristics. First, the modelled differences in atmospheric CH4 among the sites show improvement after inversion when compared to observations, implying the CH4 observation differences could help in verifying the inversion results. Second, the seasonal variations show slow onset and a late-summer maximum, indicating wetland CH4 flux has hysteretic dependence on air temperature. Third, the boreal winter natural CH4 emissions, usually treated as negligible, appear quantifiable (≥ 20 % of annual emissions). Understanding winter emission is important for climate prediction, as the winter in Canada is warming faster than the summer. Fourth, the inter-annual variability in estimated CH4 emissions is positively correlated with summer air temperature anomalies. This could enhance Canada's natural CH4 emission in the warming climate.
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