The effect of polymer stiffness on magnetization reversal of magnetorheological elastomers

Autor: Andy T. Clark, David Marchfield, Zheng Cao, Tong Dang, Nan Tang, Dustin Gilbert, Elise A. Corbin, Kristen S. Buchanan, Xuemei M. Cheng
Jazyk: angličtina
Rok vydání: 2022
Předmět:
Zdroj: APL Materials, Vol 10, Iss 4, Pp 041106-041106-7 (2022)
Druh dokumentu: article
ISSN: 2166-532X
DOI: 10.1063/5.0086761
Popis: Ultrasoft magnetorheological elastomers (MREs) offer convenient real-time magnetic field control of mechanical properties that provides a means to mimic mechanical cues and regulators of cells in vitro. Here, we systematically investigate the effect of polymer stiffness on magnetization reversal of MREs using a combination of magnetometry measurements and computational modeling. Poly-dimethylsiloxane-based MREs with Young’s moduli that range over two orders of magnitude were synthesized using commercial polymers Sylgard™ 527, Sylgard 184, and carbonyl iron powder. The magnetic hysteresis loops of the softer MREs exhibit a characteristic pinched loop shape with almost zero remanence and loop widening at intermediate fields that monotonically decreases with increasing polymer stiffness. A simple two-dipole model that incorporates magneto-mechanical coupling not only confirms that micrometer-scale particle motion along the applied magnetic field direction plays a defining role in the magnetic hysteresis of ultrasoft MREs but also reproduces the observed loop shapes and widening trends for MREs with varying polymer stiffnesses.
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