Adiabatic population transfer between electronic states of LiH molecule in two picosecond laser pulses

Autor: Ying-Yu Niu, Rong Wang
Jazyk: angličtina
Rok vydání: 2018
Předmět:
Zdroj: AIP Advances, Vol 8, Iss 11, Pp 115003-115003-12 (2018)
Druh dokumentu: article
ISSN: 2158-3226
DOI: 10.1063/1.5052465
Popis: The population transfer of stimulated Raman adiabatic passage (STIRAP) is investigated using a time-dependent quantum wave packet method. The population is transferred from an initial state to a target state through the interaction of the external laser field with the permanent dipole moment and the transition dipole moment. The laser field is composed of an infrared pulse and a near ultraviolet pulse. The two pulses with small detunings are more efficient to achieve the STIRAP transition. The process of STIRAP is sensitive to the detunings of the two pulses. When the two detunings are the same in a Λ transition or the positive detuning of the pump pulse is equal to the negative detuning of the Stokes pulse in a ladder transition, the final population in the intermediate state can be eliminated and the target population is increased.
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