Valorization of Tropical Almond ( Terminalia catappa ) Leaves into Iron-Containing Activated Carbon for Rapid Catalytic Degradation of Methylene Blue with Hydrogen Peroxide

Autor: Nhi Thi Kieu Nguyen, Duong Thi Thuy Le, Khang Dinh Vo, Linh Tung Huynh, Hung Minh Nguyen, Tuyet-Mai Tran-Thuy, Long Quang Nguyen, Dung Van Nguyen
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Journal of Ecological Engineering, Vol 25, Iss 8, Pp 54-61 (2024)
Druh dokumentu: article
ISSN: 2299-8993
22998993
DOI: 10.12911/22998993/189672
Popis: This study sought to use tropical almond leaves (TALs) for the simple fabrication of iron-containing activated carbon (IAC). Iron precursor (FeCl3) and activating agent (KOH) were sequentially preloaded in TALs. One-pot pyrolysis then generated iron-based particles (8.7 wt%), mainly metallic iron crystals, within AC support. The specific saturation magnetization of IAC was measured to be 48.9 emu/g, highlighting its ability to be efficiently separated using external magnetic fields. Moreover, the activation process yielded IAC with a large total volume of 0.28 cm3/g and a high specific surface area of 463 m2/g. Accordingly, IAC was investigated as an oxidation catalyst to degrade methylene blue (MB) by H2O2. At pH 3.0, 800 ppm H2O2, and 0.10 g/L IAC, 95.3% of MB (200 ppm) was removed after 30 min of adsorption and 60 min of oxidation. Altogether, iron-containing activated carbon from fallen leaves of tropical almonds proved its potential for robust methylene blue degradation by H2O2.
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