Strain-tuned incompatible magnetic exchange-interaction in La2NiO4

Autor: Izabela Biało, Leonardo Martinelli, Gabriele De Luca, Paul Worm, Annabella Drewanowski, Simon Jöhr, Jaewon Choi, Mirian Garcia-Fernandez, Stefano Agrestini, Ke-Jin Zhou, Kurt Kummer, Nicholas B. Brookes, Luo Guo, Anthony Edgeton, Chang B. Eom, Jan M. Tomczak, Karsten Held, Marta Gibert, Qisi Wang, Johan Chang
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Communications Physics, Vol 7, Iss 1, Pp 1-7 (2024)
Druh dokumentu: article
ISSN: 2399-3650
DOI: 10.1038/s42005-024-01701-x
Popis: Abstract Magnetic frustration is a route for novel ground states, including spin liquids and spin ices. Such frustration can be introduced through either lattice geometry or incompatible exchange interactions. Here, we find that epitaxial strain is an effective tool for tuning antiferromagnetic exchange interactions in a square-lattice system. By studying the magnon excitations in La2NiO4 films using resonant inelastic x-ray scattering, we show that the magnon displays substantial dispersion along the antiferromagnetic zone boundary, at energies that depend on the lattice of the film’s substrate. Using first principles simulations and an effective spin model, we demonstrate that the antiferromagnetic next-nearest neighbour coupling is a consequence of the two-orbital nature of La2NiO4. Altogether, we illustrate that compressive epitaxial strain enhances this coupling and, as a result, increases the level of incompatibility between exchange interactions within a model square-lattice system.
Databáze: Directory of Open Access Journals
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