High‐n Phase Suppression for Efficient and Stable Blue Perovskite Light‐Emitting Diodes

Autor: Piaoyang Shen, Shuo Ding, Zhaobing Tang, Lei Qian, Ting Zhang, Peng Xiao, Tao Chen, Hao Chen, Xinyu Zhang, Yong Ren, Dewei Zhao, Chaoyu Xiang
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Advanced Science, Vol 11, Iss 34, Pp n/a-n/a (2024)
Druh dokumentu: article
ISSN: 2198-3844
DOI: 10.1002/advs.202306167
Popis: Abstract Quasi‐2D perovskites light‐emitting diodes (PeLEDs) have achieved significant progress due to their superior optical and electronic properties. However, the blue PeLEDs still exist inefficient energy transfer and electroluminescence performance caused by mixed multidimensional phase distribution. In this work, transition metal salt (zinc bromide, ZnBr2) is introduced to modulate phase distributions by suppressing the nucleation of high n phase perovskites, which effectively shortens the energy transfer path for blue emission. Moreover, ZnBr2 also facilitates energy level matching and reduces non‐radiative recombination, thus improving electroluminescence (EL) efficiency. Benefiting from these combined improvements, an efficient blue PeLEDs is obtained with a maximum external quantum efficiency (EQE) of 16.2% peaking located at 486 nm. This work provides a promising approach to tune phase distribution of quasi‐2D perovskites and achieving highly efficient blue PeLEDs.
Databáze: Directory of Open Access Journals
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