Resonant X-ray emission spectroscopy using self-seeded hard X-ray pulses at PAL-XFEL

Autor: Tae-Kyu Choi, Jaeku Park, Gyujin Kim, Hoyoung Jang, Sang-Youn Park, Jang Hyeob Sohn, Byoung Ick Cho, Hyunjung Kim, Kyung Sook Kim, Inhyuk Nam, Sae Hwan Chun
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: Journal of Synchrotron Radiation, Vol 30, Iss 6, Pp 1038-1047 (2023)
Druh dokumentu: article
ISSN: 1600-5775
16005775
DOI: 10.1107/S1600577523007312
Popis: Self-seeded hard X-ray pulses at PAL-XFEL were used to commission a resonant X-ray emission spectroscopy experiment with a von Hamos spectrometer. The self-seeded beam, generated through forward Bragg diffraction of the [202] peak in a 100 µm-thick diamond crystal, exhibited an average bandwidth of 0.54 eV at 11.223 keV. A coordinated scanning scheme of electron bunch energy, diamond crystal angle and silicon monochromator allowed us to map the Ir Lβ2 X-ray emission lines of IrO2 powder across the Ir L3-absorption edge, from 11.212 to 11.242 keV with an energy step of 0.3 eV. This work provides a reference for hard X-ray emission spectroscopy experiments utilizing self-seeded pulses with a narrow bandwidth, eventually applicable for pump–probe studies in solid-state and diluted systems.
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