Sequential fission and the influence of 208Pb closed shells on the dynamics of superheavy element synthesis reactions

Autor: D.Y. Jeung, D.J. Hinde, M. Dasgupta, C. Simenel, E.C. Simpson, K.J. Cook, H.M. Albers, J. Buete, I.P. Carter, Ch.E. Düllmann, J. Khuyagbaatar, B. Kindler, N. Lobanov, B. Lommel, C. Mokry, E. Prasad, J. Runke, C. Sengupta, J.F. Smith, P. Thörle-Pospiech, N. Trautmann, K. Vo-Phuoc, J. Walshe, E. Williams, A. Yakushev
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: Physics Letters B, Vol 837, Iss , Pp 137641- (2023)
Druh dokumentu: article
ISSN: 0370-2693
DOI: 10.1016/j.physletb.2022.137641
Popis: Measured binary quasifission mass spectra in reactions with actinide nuclides show a large peak in yield near the doubly-magic 208Pb. This has generally been attributed to the enhanced binding energy of 208Pb causing a valley in the potential energy surface, attracting quasifission trajectories. To investigate this interpretation, binary quasifission mass spectra and cross-sections have been measured at near-barrier energies for reactions of 50Ti with actinide nuclides from 238U to 249Cf. Cross-sections have also been deduced for sequential fission (a projectile-like nucleus and two fragments from fission of the complementary target-like nucleus). Binary cross-sections fall from ∼70% of calculated capture cross-sections for 238U to only ∼40% for 249Cf, with a compensating increase in sequential fission cross-sections. The data are consistent with the 208Pb peak originating largely from sequential fission of heavier fragments produced in more mass-asymmetric primary quasifission events. These are increasingly suppressed as the heavy quasifission fragment mass increases above 208Pb. The important role of sequential fission calls for re-interpretation of quasifission characteristics and dynamics in superheavy element synthesis reactions.
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