Large-Scale Self-Assembly of anisotropic graphene oxide films via blade Coating: Sustainable design and Stimuli-Responsive performance for biomimicry

Autor: Musen Chen, Qian Wang, Maxim Trubyanov, Kou Yang, Aleksandr S. Aglikov, Ge Qi, Ekaterina V. Skorb, Kostya S. Novoselov, Daria V. Andreeva
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: Materials & Design, Vol 233, Iss , Pp 112205- (2023)
Druh dokumentu: article
ISSN: 0264-1275
DOI: 10.1016/j.matdes.2023.112205
Popis: Sustainable structural design, utilizing material to imitate natural biological systems, presents both promise and challenges. By avoiding interfacial problems encountered in composite counterparts, such designs offer self-adaptive materials for smart housing and green architecture, etc. In this study, we demonstrate the feasibility of large-scale self-assembly of graphene oxide (GO) flakes into anisotropic films through a simple blade coating technique. Through the application of blade coating to a highly concentrated nematic GO suspension, we successfully fabricate GO films with morphological gradient and patterning. Additionally, we propose a statistical analysis method utilizing scanning electron microscopy (SEM) images for the characterization of materials with macroscopic surface morphology. Furthermore, we explore the application of these GO films as low-dimensional soft actuators, revealing their outstanding stimuli-responsive performance and self-adaptation to environment. Such robust and flexible films can be used as integral building elements in the bioinspired design of sustainable smart housing facilitating remote robotization and sensing capabilities.
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