| Autor: |
Iker Gallardo, Andres Arnau, Fernando Delgado, Romana Baltic, Aparajita Singha, Fabio Donati, Christian Wäckerlin, Jan Dreiser, Stefano Rusponi, Harald Brune |
| Jazyk: |
angličtina |
| Rok vydání: |
2019 |
| Předmět: |
|
| Zdroj: |
New Journal of Physics, Vol 21, Iss 7, p 073053 (2019) |
| Druh dokumentu: |
article |
| ISSN: |
1367-2630 |
| DOI: |
10.1088/1367-2630/ab3077 |
| Popis: |
We combine x-ray absorption spectroscopy (XAS), x-ray magnetic circular dichroism (XMCD) and x-ray magnetic linear dichroism (XMLD) data with first principles density functional theory (DFT) calculations and a multiorbital many-body Hamiltonian approach to understand the electronic and magnetic properties of Co atoms adsorbed on h-BN/Ru(0001) and h-BN/Ir(111). The XAS line shape reveals, for both substrates, an electronic configuration close to 3 d ^8 , corresponding to a spin S = 1. Magnetic field dependent XMCD data show large (14 meV) out-of-plane anisotropy on h-BN/Ru(0001), while it is almost isotropic (tens of μ eV) on h-BN/Ir(111). XMLD data together with both DFT calculations and the results of the multiorbital Hubbard model suggest that the dissimilar magnetic anisotropy originates from different Co adsorption sites, namely atop N on h-BN/Ru(0001) and 6-fold hollow on h-BN/Ir(111). |
| Databáze: |
Directory of Open Access Journals |
| Externí odkaz: |
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