Inelastic Neutron Scattering Study of Phonon Dispersion Relation in Higher Manganese Silicides

Autor: Randy Belanger, James Patrick Clancy, Sheetal Jain, Zahra Yamani, Yu-Chih Tseng, Young-June Kim
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: Crystals, Vol 13, Iss 5, p 741 (2023)
Druh dokumentu: article
ISSN: 2073-4352
DOI: 10.3390/cryst13050741
Popis: We report inelastic neutron scattering (INS) measurements of the phonon dispersion relation in higher manganese silicides (HMSs). A large ingot of HMS is synthesized using a slow cooling method, which is found to have Mn15Si26 as the primary phase. The sample is composed of highly oriented crystallites as confirmed by a neutron pole-figure study and thermal conductivity data. Our INS results are mostly consistent with earlier experimental and theoretical phonon studies in HMS, including the presence of a low-lying twisting mode. However, some discrepancies are also observed. Most notably, a 5 meV gap at the zone center and the softer dispersion relation of the low-lying twisting mode. We discuss the potential origins of these observations and their implications for the thermal properties of HMS.
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