Can the remote sensing of combustion phase improve estimates of landscape fire smoke emission rate and composition?

Autor: F. Owsley-Brown, M. J. Wooster, M. J. Grosvenor, Y. Liu
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Atmospheric Measurement Techniques, Vol 17, Pp 6247-6264 (2024)
Druh dokumentu: article
ISSN: 1867-1381
1867-8548
DOI: 10.5194/amt-17-6247-2024
Popis: The proportion of flaming and smouldering (or smoldering) activity occurring in landscape fires varies with fuel type and fuel characteristics, which themselves are influenced by ecology, meteorology, time since the last fire, etc. The proportion of these combustion phases greatly influences the rate of fuel consumption and smoke emission, along with the chemical composition of the smoke, which influences the effects on the atmosphere. Earth observation (EO) has long been suggested as a way to remotely map combustion phase, and here we provide the first known attempt at evaluating whether such approaches can lead to the desired improvements in smoke emissions estimation. We use intensively measured laboratory burns to evaluate two EO approaches hypothesized to enable remote determination of combustion phase and concurrent measurements of the smoke to determine how well each is able to improve estimation of smoke emission rates, smoke composition, and the overall rate of fuel consumption. The first approach aims to estimate the sub-pixel “effective fire temperature”, which has been suggested to differ between flaming and smouldering combustion, and the second detects the potassium emission line (K-line) believed only to be present during flaming combustion. We find while the fire effective temperature approach can be suited to estimating fire radiative power (FRP), it does not significantly improve on current approaches to estimate smoke chemical makeup and smoke emission. The K-line approach does however provide these improvements when combined with the FRP data, improving the accuracy of the estimated CO2 emission rate by an average of 17±4 % and 42±15 %, respectively, depending on whether the K-line detection is used to simply classify the presence of flaming combustion or whether its magnitude is also used to estimate its relative proportion. Estimates of CO and CH4 emission rates were improved to a lesser extent than that of CO2, but the accuracy of the smoke modified combustion efficiency (MCE) estimates increased by 30±15 % and 46±10 %, respectively. MCE is correlated to the emissions factors (EFs) of many smoke constituents, so remotely deriving MCE provides a way to tailor these during smoke emissions calculations. Whilst we derived and tested our approaches on laboratory burns, we demonstrate their wider efficacy using airborne EO data of a boreal forest wildfire where we find that combined use of K-line and FRP data significantly changed estimated smoke MCE and CO2 and CO emission rates compared to the standard approach. Our findings suggest that satellite EO methods that jointly provide K-line and FRP data could enable marked improvements in the mapping of landscape fire combustion phase, fuel consumption, and smoke emissions rate and composition.
Databáze: Directory of Open Access Journals
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