Simulating exciton migration and annihilation dynamics in higher order spectroscopies of a molecular trimer

Autor: Heshmatpour Constantin, Šanda František, Lincoln Craig N., Perlík Vaclav, Malevich Pavel, Hauer Jurgen
Jazyk: angličtina
Rok vydání: 2019
Předmět:
Zdroj: EPJ Web of Conferences, Vol 205, p 06016 (2019)
Druh dokumentu: article
ISSN: 2100-014X
DOI: 10.1051/epjconf/201920506016
Popis: We present simulations of 3rd and 5th order multidimensional time-dependent signals of a molecular trimer. The developed model allows for the simulation of both signal types within one theoretical framework. We therefore extended standard Redfield theory of exciton migration by a new term to include the process of exciton-exciton annihilation.
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