Independence of optical absorption on Auger ionization in single-walled carbon nanotubes revealed by ultrafast e–h photodoping

Autor: Mitchell D Anderson, Meghan N Beattie, Jack A Alexander-Webber, Robin J Nicholas, James M Fraser
Jazyk: angličtina
Rok vydání: 2016
Předmět:
Zdroj: New Journal of Physics, Vol 18, Iss 2, p 023051 (2016)
Druh dokumentu: article
ISSN: 1367-2630
DOI: 10.1088/1367-2630/18/2/023051
Popis: Auger-ionized free-carriers in a one-dimensional semiconductor are predicted to result in a strong band-gap renormalization. Isolated single-walled carbon nanotubes (SWCNT) under high-intensity laser irradiation exhibit strong nonlinear photoluminescence (PL) due to exciton–exciton annihilation (EEA). The presence of exciton disassociation during the rapid Auger-ionization caused by EEA would lead to a strong nonlinear absorption. By simultaneously measuring SWCNT–PL and optical absorption of isolated SWCNT clusters in the PL saturation regime, we give evidence that Auger-ionized excitons do not disassociate but remain bound.
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