Universal quantum control of an atomic spin qubit on a surface

Autor: Yu Wang, Masahiro Haze, Hong T. Bui, We-hyo Soe, Herve Aubin, Arzhang Ardavan, Andreas J. Heinrich, Soo-hyon Phark
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: npj Quantum Information, Vol 9, Iss 1, Pp 1-6 (2023)
Druh dokumentu: article
ISSN: 2056-6387
DOI: 10.1038/s41534-023-00716-6
Popis: Abstract Scanning tunneling microscopy (STM) enables the bottom-up fabrication of tailored spin systems on a surface that are engineered with atomic precision. When combining STM with electron spin resonance (ESR), these single atomic and molecular spins can be controlled quantum-coherently and utilized as electron-spin qubits. Here we demonstrate universal quantum control of such a spin qubit on a surface by employing coherent control along two distinct directions, achieved with two consecutive radio-frequency (RF) pulses with a well-defined phase difference. We first show transformations of each Cartesian component of a Bloch vector on the quantization axis, followed by ESR-STM detection. Then we demonstrate the ability to generate an arbitrary superposition state of a single spin qubit by using two-axis control schemes, in which experimental data show excellent agreement with simulations. Finally, we present an implementation of two-axis control in dynamical decoupling. Our work extends the scope of STM-based pulsed ESR, highlighting the potential of this technique for quantum gate operations of electron-spin qubits on a surface.
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