Competition between orbital effects, Pauli limiting, and Fulde–Ferrell–Larkin–Ovchinnikov states in 2D transition metal dichalcogenide superconductors

Autor: Chang-woo Cho, Cheuk Yin Ng, Chi Ho Wong, Mahmoud Abdel-Hafiez, Alexander N Vasiliev, Dmitriy A Chareev, A G Lebed, Rolf Lortz
Jazyk: angličtina
Rok vydání: 2022
Předmět:
Zdroj: New Journal of Physics, Vol 24, Iss 8, p 083001 (2022)
Druh dokumentu: article
ISSN: 1367-2630
DOI: 10.1088/1367-2630/ac8114
Popis: We compare the upper critical field of bulk single-crystalline samples of the two intrinsic transition metal dichalcogenide superconductors, 2H-NbSe _2 and 2H-NbS _2 , in high magnetic fields where their layer structure is aligned strictly parallel and perpendicular to the field, using magnetic torque experiments and a high-precision piezo-rotary positioner. While both superconductors show that orbital effects still have a significant impact when the layer structure is aligned parallel to the field, the upper critical field of NbS _2 rises above the Pauli limiting field and forms a Fulde–Ferrell–Larkin–Ovchinnikov (FFLO) state, while orbital effects suppress superconductivity in NbSe _2 just below the Pauli limit, which excludes the formation of the FFLO state. From the out-of-plane anisotropies, the coherence length perpendicular to the layers of 31 Å in NbSe _2 is much larger than the interlayer distance, leading to a significant orbital effect suppressing superconductivity before the Pauli limit is reached, in contrast to the more 2D NbS _2 .
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