Ultralow Threshold Room Temperature Polariton Condensation in Colloidal CdSe/CdS Core/Shell Nanoplatelets

Autor: Hongyu Yang, Lei Zhang, Wenbin Xiang, Changgui Lu, Yiping Cui, Jiayu Zhang
Jazyk: angličtina
Rok vydání: 2022
Předmět:
Zdroj: Advanced Science, Vol 9, Iss 18, Pp n/a-n/a (2022)
Druh dokumentu: article
ISSN: 2198-3844
DOI: 10.1002/advs.202200395
Popis: Abstract Room‐temperature exciton‐polariton Bose‐Einstein condensation (BEC), a phase transition to single quantum state with strong nonlinearity, provides a new strategy for coherent light sources and ultralow threshold optic switches. In this work, colloidal CdSe/CdS 2D nanoplatelets are embedded into a microcavity, and exciton‐polariton BEC is realized with an ultralow threshold of 0.5 µJ cm–2 at room temperature. The superlinear power‐dependent emission, macroscopic occupation of the ground state, strong blueshift and broadening of the emission peak, and long‐range coherence strongly confirm the realization of the polariton laser. This work suggests considerable prospects for colloidal nanoplatelets in low‐cost, high‐performance polariton devices, and coherent light sources.
Databáze: Directory of Open Access Journals
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