Experimental observation of spin−split energy dispersion in high-mobility single-layer graphene/WSe2 heterostructures

Autor: Priya Tiwari, Mohit Kumar Jat, Adithi Udupa, Deepa S. Narang, Kenji Watanabe, Takashi Taniguchi, Diptiman Sen, Aveek Bid
Jazyk: angličtina
Rok vydání: 2022
Předmět:
Zdroj: npj 2D Materials and Applications, Vol 6, Iss 1, Pp 1-6 (2022)
Druh dokumentu: article
ISSN: 2397-7132
DOI: 10.1038/s41699-022-00348-y
Popis: Abstract Proximity-induced spin–orbit coupling in graphene has led to the observation of intriguing phenomena like time-reversal invariant $${{\mathbb{Z}}}_{2}$$ Z 2 topological phase and spin-orbital filtering effects. An understanding of the effect of spin–orbit coupling on the band structure of graphene is essential if these exciting observations are to be transformed into real-world applications. In this research article, we report the experimental determination of the band structure of single-layer graphene (SLG) in the presence of strong proximity-induced spin–orbit coupling. We achieve this in high-mobility hexagonal boron nitride (hBN)-encapsulated SLG/WSe2 heterostructures through measurements of quantum oscillations. We observe clear spin-splitting of the graphene bands along with a substantial increase in the Fermi velocity. Using a theoretical model with realistic parameters to fit our experimental data, we uncover evidence of a band gap opening and band inversion in the SLG. Further, we establish that the deviation of the low-energy band structure from pristine SLG is determined primarily by the valley-Zeeman SOC and Rashba SOC, with the Kane–Mele SOC being inconsequential. Despite robust theoretical predictions and observations of band-splitting, a quantitative measure of the spin-splitting of the valence and the conduction bands and the consequent low-energy dispersion relation in SLG was missing—our combined experimental and theoretical study fills this lacuna.
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