Nonlinear mid-infrared meta-membranes

Autor: Sartorello Giovanni, Bocanegra Joshua, Knez David, Lukin Daniil M., Yang Joshua, Vučković Jelena, Fishman Dmitry A., Shvets Gennady, Shcherbakov Maxim R.
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: Nanophotonics, Vol 13, Iss 18, Pp 3395-3402 (2024)
Druh dokumentu: article
ISSN: 2192-8614
DOI: 10.1515/nanoph-2024-0203
Popis: Nanophotonic structures have shown promising routes to controlling and enhancing nonlinear optical processes at the nanoscale. However, most nonlinear nanostructures require a handling substrate, reducing their application scope. Due to the underwhelming heat dissipation, it has been a challenge to evaluate the nonlinear optical properties of free-standing nanostructures. Here, we overcome this challenge by performing shot-controlled fifth harmonic generation (FHG) measurements on a SiC meta-membrane – a free-standing transmission metasurface with pronounced optical resonances in the mid-infrared (λ res ≈ 4,000 nm). Back focal plane imaging of the FHG diffraction orders and rigorous finite-difference time-domain simulations reveal at least two orders of magnitude enhancement of the FHG from the meta-membrane, compared to the unstructured SiC film of the same thickness. Single-shot measurements of the meta-membrane with varying resonance positions reveal an unusual spectral behavior that we explain with Kerr-driven intensity-dependent resonance dynamics. This work paves the way for novel substrate-less nanophotonic architectures.
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