High enrichment of heavy metals in fine particulate matter through dust aerosol generation
| Autor: | Q. Gao, S. Zhu, K. Zhou, J. Zhai, S. Chen, Q. Wang, S. Wang, J. Han, X. Lu, H. Chen, L. Zhang, L. Wang, Z. Wang, X. Yang, Q. Ying, H. Zhang, J. Chen, X. Wang |
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| Jazyk: | angličtina |
| Rok vydání: | 2023 |
| Předmět: | |
| Zdroj: | Atmospheric Chemistry and Physics, Vol 23, Pp 13049-13060 (2023) |
| Druh dokumentu: | article |
| ISSN: | 1680-7316 1680-7324 |
| DOI: | 10.5194/acp-23-13049-2023 |
| Popis: | Dust is a major source of atmospheric aerosols. Its chemical composition is often assumed to be similar to the parent soil. However, this assumption has not been rigorously verified. Here, we generated dust aerosols from soils to determine if there is particle-size-dependent selectivity of heavy metals in the dust generation. Mn, Cd, Pb and other heavy metals were found to be highly enriched in fine-dust (PM2.5) aerosols, which can be up to ∼ 6.5-fold. To calculate the contributions of dust to atmospheric heavy metals, regional air quality models usually use the dust chemical profiles from the U.S. Environmental Protection Agency's (EPA) SPECIATE database, which does not capture the correct size-dependent selectivity of heavy metals in dust aerosols. Our air quality modeling for China demonstrates that the calculated contribution of fine-dust aerosols to atmospheric heavy metals, as well as their cancer risks, could have significant errors without using proper dust profiles. |
| Databáze: | Directory of Open Access Journals |
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