Autor: |
Ma, Qianli, Billingsley, Brianna R., Marshall, Madalynn, Dahlbom, David A., Hao, Yiqing, Pajerowski, Daniel M., Kolesnikov, Alexander I., Bai, Xiaojian, Batista, Cristian D., Kong, Tai, Cao, Huibo |
Rok vydání: |
2024 |
Předmět: |
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Druh dokumentu: |
Working Paper |
Popis: |
We report a comprehensive study on the origin of the enigmatic disordered ground state within the Shastry-Sutherland lattice, BaCe$_2$ZnS$_5$, at low temperatures. The magnetization and heat capacity data show a lack of magnetic ordering down to 73 mK. We deploy a localized spin dimer model which can accurately reproduce the dynamic structure factor of the neutron data, magnetization and heat capacity data. Remarkably, the intra-dimer exchange interaction shows strong XY-type anisotropy and the ground state of BaCe$_2$ZnS$_5$ is in an entangled state $(|\uparrow\uparrow> - |\downarrow\downarrow>)/\sqrt{2}$. This is in contrast to the singlet dimer state that is obtained for Heisenberg interactions. These results confirm that BaCe$_2$ZnS$_5$ is in a quantum paramagnet state consisting of entangled spin dimer states. |
Databáze: |
arXiv |
Externí odkaz: |
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