Closing of the Mott gap near step edges in NiS2

Autor: Yasui, Yuuki, Iwata, Kota, Okazaki, Shota, Miyasaka, Shigeki, Sugimoto, Yoshiaki, Hanaguri, Tetsuo, Takagi, Hidenori, Sasagawa, Takao
Rok vydání: 2024
Předmět:
Zdroj: Phys. Rev. B 110, 045139 (2024)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.110.045139
Popis: A prototypical charge-transfer type Mott insulator NiS2 pyrite exhibits a metal-insulator transition with bandwidth control. Recent discoveries on surface-specific electronic states on other 3d transition-metal disulfide pyrites motivate us to further investigate the surface of NiS2, where metallic surface conduction is discussed. Here, the spectroscopic-imaging scanning-tunneling-microscopy observations revealed that the surface is not metallic, contrary to the expectation. Instead, the Mott gap is closed near step edges, suggesting possible electrical conduction from one-dimensional channels. The edge anomaly was observed irrespective of its magnetic order and is limited to the insulator phases.
Comment: 5 pages, 5 figures
Databáze: arXiv