| Popis: |
We identify common features, seen across a wide range of actinide and lanthanide based heavy-fermion metals, that we associate with the universal properties of the residual moments generated by Kondo hybridisation. The features include the opposing anisotropies of the effective moments and Curie-Weiss constants, the reorientation of the magnetic easy axis, the hard-axis susceptibility maximum and the hard-axis metamagnetic transition. The extension of large-$N$ Read-Newns theory to the underscreened Kondo lattice allows us to study large magnetic fluctuations of residual local moments in the presence of strong $f$-$d$ hybridisation. We derive an effective Hamiltonian for the residual moments and show that competing single-ion and exchange anisotropies are responsible for the easy-axis reorientation. We identify a strong-coupling regime, where the temperature of the easy-axis reorientation is {\it directly proportional} to the coherence temperature and find good agreement across several Eu and U based heavy-fermion families, as well as a weak-coupling regime, where the easy axis flips just before the onset of magnetic order, as is seen in many Ce and Yb heavy-fermion compounds. We show that the exchange anisotropy of the residual moments can also generate a maximum in the hard-axis susceptibility, and find good agreement with UTe$_2$ at low pressures, suggesting that this material is particularly well described by the single-channel $S=1$ model. Finally, we speculate on the possible pairing interactions generated by the fluctuations of the residual moments. |
