Large magnetoresistance and first-order phase transition in antiferromagnetic single-crystalline EuAg$_4$Sb$_2$
| Autor: | Malick, Sudip, Świątek, Hanna, Bławat, Joanna, Singleton, John, Klimczuk, Tomasz |
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| Rok vydání: | 2024 |
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| Zdroj: | Phys. Rev. B 110, 165149 (2024) |
| Druh dokumentu: | Working Paper |
| DOI: | 10.1103/PhysRevB.110.165149 |
| Popis: | We present the results of a thorough investigation of the physical properties of EuAg$_4$Sb$_2$ single crystals using magnetization, heat capacity, and electrical resistivity measurements. High-quality single crystals, which crystallize in a trigonal structure with space group $R\bar{3}m$, were grown using a conventional flux method. Temperature-dependent magnetization measurements along different crystallographic orientations confirm two antiferromagnetic phase transitions around $T_{N1}$ = 10.5 K and $T_{N2}$ = 7.5 K. Isothermal magnetization data exhibit several metamagnetic transitions below these transition temperatures. Antiferromagnetic phase transitions in EuAg$_4$Sb$_2$ are further confirmed by two sharp peaks in the temperature-dependent heat capacity data at $T_{N1}$ and $T_{N2}$, which shift to the lower temperature in the presence of an external magnetic field. Our systematic heat capacity measurements utilizing a long-pulse and single-slope analysis technique allow us to detect a first-order phase transition in EuAg$_4$Sb$_2$ at 7.5 K. The temperature-dependent electrical resistivity data also manifest two features associated with magnetic order. The magnetoresistance exhibits a broad hump due to the field-induced metamagnetic transition. Remarkably, the magnetoresistance keeps increasing without showing any tendency to saturate as the applied magnetic field increases, and it reaches $\sim$20000\% at 1.6 K and 60 T. At high magnetic fields, several magnetic quantum oscillations are observed, indicating a complex Fermi surface. A large negative magnetoresistance of about -55\% is also observed near $T_{N1}$. Moreover, the $H$-$T$ phase diagram constructed using magnetization, heat capacity, and magnetotransport data indicates complex magnetic behavior in EuAg$_4$Sb$_2$. Comment: 10 pages, 6 figures |
| Databáze: | arXiv |
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