Large band-splitting in $g$-wave type altermagnet CrSb

Autor: Ding, Jianyang, Jiang, Zhicheng, Chen, Xiuhua, Tao, Zicheng, Liu, Zhengtai, Liu, Jishan, Li, Tongrui, Liu, Jiayu, Yang, Yichen, Zhang, Runfeng, Deng, Liwei, Jing, Wenchuan, Huang, Yu, Shi, Yuming, Qiao, Shan, Wang, Yilin, Guo, Yanfeng, Feng, Donglai, Shen, Dawei
Rok vydání: 2024
Předmět:
Druh dokumentu: Working Paper
Popis: Altermagnetism (AM), a newly discovered magnetic state, ingeniously integrates the properties of ferromagnetism and antiferromagnetism, representing a significant breakthrough in the field of magnetic materials. Despite experimental verification of some typical AM materials, such as MnTe and MnTe$_2$, the pursuit of AM materials that feature larger spin splitting and higher transition temperature is still essential. Here, our research focuses on CrSb, which possesses N{\'e}el temperature of up to 700K and giant spin splitting near the Fermi level ($E_F$). Utilizing high-resolution angle-resolved photoemission spectroscopy and density functional theory calculations, we meticulously map the three-dimensional electronic structure of CrSb. Our photoemission spectroscopic results on both (0001) and (10$\overline{1}$0) cleavages of CrSb collaboratively reveal unprecedented details on AM-induced band splitting, and subsequently pin down its unique bulk $g$-wave symmetry through quantitative analysis of the angular and photon-energy dependence of spin splitting. Moreover, the observed spin splitting reaches the magnitude of 0.93~eV near $E_F$, the most substantial among all confirmed AM materials. This study not only validates the nature of CrSb as a prototype $g$-wave like AM material but also underscores its pivotal role in pioneering applications in spintronics.
Databáze: arXiv