| Autor: |
Mardelé, Florian le, Mohelský, Ivan, Wyzula, Jan, Orlita, Milan, Turek, Philippe, Troiani, Filippo, Boudalis, Athanassios K. |
| Rok vydání: |
2024 |
| Předmět: |
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| Druh dokumentu: |
Working Paper |
| Popis: |
Electric fields represent an ideal means for controlling spins at the nanoscale and, more specifically, for manipulating protected degrees of freedom in multispin systems. Here we perform low-temperature magnetic far-IR spectroscopy on a molecular spin triangle (Fe3) and provide the first experimental evidence of spin-electric transitions in polynuclear complexes. The co-presence of electric- and magnetic-dipole transitions, allows us to estimate the spin-electric coupling. Based on spin Hamiltonian simulations of the spectra, we identify the observed transitions and introduce the concept of a generalized exchange qubit. This applies to a wide class of molecular spin triangles, and includes the scalar chirality and the partial spin sum qubits as special cases. |
| Databáze: |
arXiv |
| Externí odkaz: |
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