Magneto-synthesis effect on magnetic order, phonons, and magnons in single-crystal Sr$_2$IrO$_4$

Autor: Pellatz, Nicholas, Kim, Jungho, Kim, Jong-Woo, Kimchi, Itamar, Cao, Gang, Reznik, Dmitry
Rok vydání: 2024
Předmět:
Zdroj: Phys. Rev. Materials 7, 123802 (2023)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevMaterials.7.123802
Popis: It was shown earlier that applying a magnetic field during the growth of Sr$_2$IrO$_4$, also known as "field-alteration", induces significant changes to its structural, magnetic, and transport properties. However, the microscopic nature of these changes is enigmatic. In this study, we employed resonant elastic and inelastic x-ray scattering, as well as Raman scattering, to investigate samples from two batches of Sr$_2$IrO$_4$ grown in magnetic fields of different strengths. Our findings reveal that samples grown in a weaker magnetic field have similar magnetic order to non-altered samples, whereas those grown in a stronger field show a different stacking of weak in-plane ferromagnetic moments. Additionally, we observed significant softening and broadening of select Raman-active phonons in the field altered samples, with a stronger effect in the samples grown in the stronger field. We discuss insights that our results provide into the microscopic nature of field-alteration in Sr$_2$IrO$_4$.
Databáze: arXiv