Three-photon electron spin resonances
| Autor: | Atwood, S. I., Mkhitaryan, V. V., Dhileepkumar, S., Nuibe, C., Hosseinzadeh, S., Malissa, H., Lupton, J. M., Boehme, C. |
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| Rok vydání: | 2023 |
| Předmět: | |
| Zdroj: | Phys. Rev. B 110, L060103 (2024) |
| Druh dokumentu: | Working Paper |
| DOI: | 10.1103/PhysRevB.110.L060103 |
| Popis: | We report the observation of a three-photon resonant transition of charge-carrier spins in an organic light-emitting diode using electrically detected magnetic resonance (EDMR) spectroscopy at room temperature. Under strong magnetic-resonant drive (drive field $B_1$ ~ static magnetic field $B_0$), a $B_0$-field swept EDMR line emerges when $B_0$ is approximately threefold the one-photon resonance field. Ratios of drive-induced shifts of this line to those of two- and one-photon shifts agree with analytical expressions derived from the Floquet Hamiltonian and confirm the nature of these three-photon transitions, enabling access of spin physics to a hitherto inaccessible domain of quantum mechanics. Comment: 32 pages, 18 figures |
| Databáze: | arXiv |
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